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Код

private Dictionary<double, double> GetArrangement(double noiseLevel)
        {
            double lowest = ConvertDataPoint(currentChart.Series[0].Points.FindMinByValue());
            double highest = ConvertDataPoint(currentChart.Series[0].Points.FindMaxByValue());

            double current = lowest;

            List<double> x = new List<double>();    //Значения

            Dictionary<double, double> arrangementTable = new Dictionary<double, double>();

            while(current<=highest)
            {
                x.Add(current);
                current += noiseLevel;
            }

            List<int> p = new List<int>(); //Вероятности
            for (int i = 0; i < x.Count; i++)
            {
                p.Add(0);
            }
            for (int i = 0; i < x.Count; i++)
                {
                    for (int j = 0; j < currentChart.Series[0].Points.Count; j++)
                    {
                        if (Math.Abs(x[i] - ConvertDataPoint(currentChart.Series[0].Points[j])) <= noiseLevel)
                        {
                            p[i] += 1;
                        }
                    }
                    arrangementTable.Add(x[i], p[i]);  //Изменена коллекция
                }

            int total = 0;
            foreach(KeyValuePair<double, double> item in arrangementTable)  //ИСКЛЮЧЕНИЕ
            {
                total += (int)item.Value;
            }

            foreach (KeyValuePair<double, double> item in arrangementTable)
            {
                arrangementTable[item.Key] = (item.Value*100)/total;
            }

            return arrangementTable;
        }